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Creators/Authors contains: "Seguin, Trevor J."

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  1. ; ; ( , ACS Catalysis)
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  2. ; ; ; ; ; ; ; ; ; ; et al ( , RSC Advances)
    The solvation shell structures of Ca 2+ in aqueous and organic solutions probed by calcium L-edge soft X-ray absorption spectroscopy (XAS) and DFT/MD simulations show the coordination number of Ca 2+ to be negatively correlated with the electrolyte concentration and the steric hindrance of the solvent molecule. In this work, the calcium L-edge soft XAS demonstrates its sensitivity to the surrounding chemical environment. Additionally, the total electron yield (TEY) mode is surface sensitive because the electron penetration depth is limited to a few nanometers. Thus this study shows its implications for future battery studies, especially for probing the electrolyte/electrode interface for electrochemical reactions under in situ /operando conditions. 
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  3. ; ; ; ( , Accounts of Chemical Research)